Season 5 Episode 16 - "I want this"
This was so close to making the list. Almost as satisfying as Walt admitting he never did what he did for the family. Right after killing Todd, Jesse has the chance to kill Walt, but tells him to admit that he wants to die. Walt tells Jesse he wants this (to die), but Jesse refuses to give him that pleasure of dying. Walt’s long-suffering surrogate son does see Mr. White’s mortal wound, so he realizes that Walt is going to die anyways in the end.
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